放射化学 第 27 号 - Japan Society of Nuclear and Radiochemical
Contents
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13. Amemiya Y amp Miyahara J Imaging plate illuminates many fields Nature 336 89 90 1988 HER ta Y Hi 2 Vol 45 No 6 398 404 1990 HAER WER SML X 2 3 27 47 2015 MAR ae 28 350 356 1986 4 Cesar L J et al Artefacts found in computed radiography The British Journal of Radiology 74 195 202 2001 5 Yasunari T J et al Cesium 137 deposition and contamination of Japanese soils due to the Fukushima nuclear accident PINAS 108 49 19530 19534 2
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139. 0 Measurements of Capture Gamma Rays from the Neutron Resonances of Se and Se at PARC MLF ANNRI A B amp E Measurements of Neutron Capture Cross Section for Se Se and Se at KURRI LINAC Correlation Between Asian Dust yellow dust and Specific Radioactivities of Fission Products Including in Airborne Samples in Tokushima Shikoku Island Japan due to the Fukushima Nuclear Accident Material Activation Benchmark Experiments at the NuMI Hadron Absorber Hall in Fermilab KU d Measurements of Neutron Cross Sections for Chromium Yttrium and Terbium at 197 MeV proceedings Nuclear Data Sheet
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144. 1 Nuclear Emergency Response Headquarters Government of Japan Available at http www kantel go jp foreign kan topics 201106 iaea_ houkokusho e html 2013 2 28 2011 M Chino H Nakayama H Nagai H Terada G Katata H Yamazawa J Nucl Sci Technol 48 1129 2011 N Kinoshita K Sueki K Sasa J Kitagawa o Ikarashi T Nishimura Y Wong Y Satou K Handa T Takahashi M Sato T Yamagata PNAS 108 19526 2011 N Yoshida Y Takahashi Elements 8 201 2012 o Endo 5 Kimura T Takatsuji K Nanasawa T Imanaka K Shizuma J Environ Radioact 111 18 2012 E Cardis A Kesminiene V Ivanov I Malakhova Y Shibata V Khrouch et al J National Cancer Inst 97 724 2005 K Tanaka A Sakaguchi Y Kanai H Tsuruta A Shinohara Y Takahashi J Radioanal Nucl Chem 295 1927 2013 K Tanaka Y Takahashi A Sakaguchi M Umeo S Hayakawa H Tanida T Saito Y Kanai Geochem J 46 73 2012 2 3 4 5 6 7 8 27 18 2015 9 H Kato Y Onda M Teramage J Environ Radioact 111 59 2012 10 T Ohno Y Muramatsu Y Miura K Oda N Inagawa H Ogawa A Yamazaki C Toyama M Sato Geochem J 46 287 2012 11 K Bunzl W Schimmack K Kreutzer R Schierl Sci Total Environ 78 77 1989 12 I A Scotti S Silva J Environ Radioact
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221. 16 97 1992 13 K Tanaka H Iwatani A Sakaguchi Y Takahashi Y Onda J Radioanal Nucl Chem 295 2007 2013 14 Q H Fan Y Takahashi K Tanaka A Sakaguchi An EXAFS Study on the Effect of Mineralogy Composition and Natural Organic Matter on Cesium Adsorption and Mobility Submitted to Geochim Cosmochim Acta under review 15 82 408 2011 16 B C Bostick M A Vairavamurthy K G Karthikeyan J Chorover Environ Sci Technol 36 2670 2002 17 H Qin Y Yokoyama Q Fan H Iwatani K Tanaka A Sakaguchi Y Kanai J Zhu Y Onda Y Takahashi Geochem J 46 297 2012 Abstract Various kinds of natural samples such as aerosols rock soil tree leaves and river suspended sediment were collected after the Fukushima Daiichi Nuclear Power Plant FDNPP accident Analysis of radiocesium for these samples gave us important information to discuss the post event behavior and transportation of radiocesium in the environment from the air into ground and river systems Only a small amount of airborne particles containing high radiocesium concentration which contained water soluble fractions of radiocesium were transported
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229. biphenyl bpp AT OFZ bpa bpp HET TAAFOdEE 1 Gutlich P Bill E Trautwein A L Mossbauer Spectroscopy and Transition Metal Chemistry Springer 2011 2001 Radioisotopes accepted 2013 Morita T Asada Y Okuda T Nakashima S Isomerism of Assembled Iron Complex Bridged by 1 2 Di 4 pyridyl ethane and Its Solid to Solid Transformation Accompanied by a Change of E
230. in Be C and PF nuclei between 04 and 1 9 GeV Nucl Phys A352 1981 461 476 5 Shibata and P J Karol Identification of 26 minute Zr 84 Can J Chem 61 1983 704 756 S Shibata et al Absolute g ray abundance of Zr Radiochim Acta 46 1989 1 3 S Shibata et al Photonuclear spallation reactions in Cu Phys Rev C 35 1987 254 262 K Sakamoto et al Barium and xenon 3 4 5 6 isotope yields in photopion reactions of SSCs Phys Rev C 42 1990 1545 1558 7 S Shibata et al Yield measurements of Be and Be produced by photonuclear reactions at intermediate energies Intercomparison of fragmentation processes between photon and proton induced reactions Radiochim Acta 80 1998 181 187 S R Sarkar et al Photospallation of complex nuclei at intermediate energies 8 III Comparison with PICA calculation Radiochim Acta 62 1993 7 16 9 S Shibata et al Measurements of Be and A production cross sections with 12 GeV protons by accelerator mass spectrometry Phys Rev C 48 1993 2617 2624 10 Y Uwamino et al High energy p Li neutron field for activation experiment Nucl Instr Meth Phys Res A389 1997 463 413 27 20 2015 11 S Shibata et al Measurements of the production cross sections of tritium from oxygen using p Be and p Li neutrons up to E 38 MeV Radiochim Acta 75 1996 1 6 12 S Sekimoto et al Measurement of
231. neutron cross sections for yttrium and terbium at 285 MeV Prog Nucl Sci Tech 1 2011 89 93 13 LB Ik 45 1990 178 184 14 S Shibata et al Large sized and highly radioactive H and Cd Langmuir Blodgett films Nucl Instr Meth Phys Res A350 1994 263 274 15 H Kawakami et al Precise measurement of Ag KLL Auger spectrum Phys Lett A 121 1987 414 418 16 H Kawakami et al New upper bound on the electron anti neutrino mass Phys Lett B 256 1991 105 111 17 T Ohshima et al No 17 keV neutrino Admixture lt 0 07396 95 C L Phys Rev D 47 1993 4840 4856 18 T Shibata et al A method to estimate the fast neutron fluence for the Hiroshima atomic bomb J Phys Soc Jpn 63 1994 3046 3947 19 K Takamiya et al Excitation function for Cu np 9Ni reaction in neutron energy range up to 15 MeV Appl Radiat Isot 66 2008 1321 1324 20 SNI 32 2006 146 154 21 S Shibata et al Measurement of Ni produced in Cu samples by the Hiroshima atomic bomb J Radioanal Nucl Chem 273 2007 517 520 22 K Takamiya et al Preparation of multitracer by thermal neutron fission of 25
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235. 2 May 2013 17 May 2013 Jeju South Korea http www isrs2013 0rg 2 2013 GRC NuChem 2013 Gordon Research Conference on Nuclear Chemistry 09 Jun 2013 14 Jun 2013 New London NH United States http www grc org programs aspx year 2013 amp program nuchem 3 CHES 8th Workshop on the Chemistry of the Heaviest Elements 19 Sep 2013 21 Sep 2013 Takayama Japan http asrcjaea go p CHES 4 ARCEBS 2014 Third International Conference on Application of RadiotraCers and Energetic Beams in Sciences 12 Jan 2014 18 Jan 2014 Kolkata India http indico cern ch conferenceDisplay py confld 232042 5 Actinides 2013 21 July 2013 gt 26 July 2013 Karlsruhe Germany http actinides13 ine kit edu 24 php 6 Migration conference 2013 14th International Conference on the Chemistry and Migration Behaviour of Actinides and Fission Products in the Geosphere 8 Sep 2013 13 Sep 2013 Brighton United Kingdom http www boro ac uk departments chemistry migrationconference2013 7 10th International Conference on Tritium Science and Technology TRITIUM 2013 October 21 25 2013 Nice Acropolis France http www fusion magnetique ceafr tritium2013 8 50 2013 7 3 OK 7 5
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249. che anti gauche gauche gauche Energy 2013 Dp 9 11 benzene bpp Fe NCS bpp anti anti anti gauche anti gauche gauche gauche Fe NCS bpp 2 benzene anti gauche anti gauche 1 1 1 anti gauche 2E Fe NCS bpp 2 benzene 4 bpp 44E Fe NCS bpp 4bpp 5A E 7 6 NCSe NCBH tk Fe NCX bpp X Se BH Fe NCX bpp 2 2 benzene X Se BH 4 bpp 64 Eao 4 bpp 44E
250. d by desorption and adsorption of guest benzene molecules in Fe NCS bpp 2 benzene bpp 1 3 bis 4 pyridyl propane Inorg Chim Acta 370 82 88 2011 Abstract Assembled coordination complexes have a variety of assembled structures depending on the bridging ligand When the bridging ligand is flexible more variety of assembled structure is expected depending on the conformer of the ligand 1 2 Bis 4 pyridyl ethane bpa has anti gauche conformer and 1 3 bis 4 pyridyl propane A variety of assembled structures were obtained bpp has more variety of conformer by changing conformer of bpa The appearance of spin crossover phenomenon by enclathrating guest molecule in the assembled complexes of bpa was introduced The assembled complex Fe NCBH3 s bpa 9 biphenyl was synthesized the skeleton of which was a 1D chain Several 27 11 2013 pp 3 11 1D chains gathered together to form 1D The 1D chain sheet was stacked spirally to form novel spiral assembly The chain sheet assembly showed a stepwise spin crossover phenomenon The reversible structural change of host framework triggered by desorption and adsorption of guest benzene molecules was also introduced in bpp complexes 27 2013 C w 9 sh IEIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIIEIIIIIIIIIIIIIIIIIII
251. lectronic State Bull Chem Soc Jpn 79 738 744 2006 Morita T Nakashima S Yamada K Inoue K Occurrence of the spin crossover 2 3 4 5 phenomenon of assembled complexes Fe NCX bpa X S BH bpa 12 27 10 2015 bis 4 pyridyl ethane by enclathrating organic guest molecule Chem Lett 35 1042 1043 2006 Nakashima S Morita T Inoue K Spin crossover phenomenon of the assembled 6 iron complexes with 1 2 bis 4 pyridyl ethane as bridging ligand studied by M ssbauer spectroscopy Hyperfine Interactions 188 107 111 2009 Nakashima S Morita T Inoue K and Hayam S Spiral Assembly of the 1D Chain Sheet of Fe NCBH bpa biphenyl bpa 1 2 bis 4 pyridyl ethane and its Stepwise Spin Crossover Phenomenon Polymers 4 880 888 2012 Bauer W Pfaffeneder T Achterhold K Weber B Complete two step spin 7 8 transition in a 1D chain iron II complex with a 110 K wide intermediate plateau Eur J Inorg Chem 2011 3183 3192 Atsuchi M Higashikawa H Yoshida Y Nakashima S Inoue K Novel 2D interpenetrated structure and occurrence 9 of the spin crossover phenomena of assembled complexes Fe NCX bpp X S Se BH bpp 1 3 bis 4 pyridyl propane Chem Lett 36 1064 1065 2007 10 Atsuchi M Inoue K Nakashima S Reversible structural change of host framework triggere
252. o te O t O te O lt o O lt o O lt o O lt o Oo fte O t O te O ae O O O Oo O eo e 4 O O ow o e o e o Se o fe o fe o 9e o 9e o Se o efe o fe o 9e 0 9e o 0 o fe o Se oe o 9e o efe o efe o fe oe oe o 0 o fe o 40 o 9e 0 Se o 0 o fe oe oe 0 0 o fe Es 2012 56 2012 56 2012 10 3 5 AH EK
253. onaga T Donohue D Aigner H Burger S Klose D Karkela T ZilliacusR Auvinen A Marie O PointurierF Production and Characterization of Plutonium Dioxide Particles as Quality Control Material for Safeguards Purposes Analytical Chemistry 84 2638 2646 2012 11 New Brunswick Laboratory Certified Reference Material CRM 137 Illinois October 1 1987 12 Keegan R P GehrkeR J A method to determine the time since last purification of weapons grade plutonium J Appl Radi Isot 59 137 143 2003 13 WalleniusM TomboriniG KochL The age of plutonium particles Radiochim Acta 89 55 2001 14 NygrenU RamebackH NilssonC Age determination of plutonium using inductively coupled plasma mass spectrometry J Radioanal Niucl Chem 212 4551 2007 15 New Brunswick Laboratory Certified Reference Material CRM 136 Argonne Illinois October 1 1987 goo E I
254. ura Eds KEK Proceedings 2012 6 pp 25 33 High Energy Accelerator Research Organization 2012 D 1 94 1941 Glenn T Seaborg Uranium Neptunium Plutonium Uranus EH Neptune Pluto
255. with non radioactive aerosols in the air Subsequent interaction of such water soluble fraction with water e g rainfall dissolved and strongly fixed the radiocesium on rock and soil particles clay minerals thus changing the radiocesium into insoluble forms The distribution of radiocesium was possibly controlled by the initial position of deposition from the air to the ground producing the heterogeneous distribution Such heterogeneity In river suspended particles was also observed during water transportation reflecting the heterogeneity of radiocesium in rock and soil Leaching experiments demonstrated that radiocesium in rock soil 2 8 19 2013 pp 12 19 and river suspended sediment was fairly insoluble possibly due to the formation of inner sphere complexes in clay minerals Leaching experiments also demonstrated that radiocesium in contaminated tree leaves strongly fixed in leaf tissues and is not readily released The micro scale heterogeneous distribution of radiocesium in aerosols soil and suspended particles was due to the presence of small particles in aerosols containing high radiocesium concentration Dissolution of radiocesium in the aerosol particles and subsequent irreversible adsorption onto the soil particle complex are responsible for the preservation of the heterogeneity both in soil and in river suspended particles OOO QOQQOQOQOQQQOQOQOO0QQOQ2 Q 1
256. x m S 4 J 2 S on re X 0 D LA e P 5 r 8 A s a gt e g A Ej 7 Y an 4 x y X v J x L4 27 2013 NCBH Fe NCS bpp 2 benzene bpp Fe Fe 11 675 A Fe Fe 9551 A Fe Fe 14 569 A 15 782 A 8 2
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